大科学装置专刊

短波自由电子激光在原子分子和团簇中的应用

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  • ①中国科学院上海高等研究院 基础交叉中心,上海 201210;②中国科学院大学 未来技术学院,北京 100049; ③上海科技大学 大科学中心/物质科学与技术学院,上海 201210

王新成,研究方向:原子分子光物理的实验和理论研究。

江玉海,研究方向:原子分子以及纳米材料光物理的实验和理论研究。

收稿日期: 2024-03-05

  网络出版日期: 2024-06-27

基金资助

国家重点研发计划课题(2022YFA1604302)和国家自然科学基金重点项目(12334011)

Atomic, molecular and cluster applications of short-wavelength free-electron lasers

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  • ① Shanghai Advanced Research Institute, Chinese Academy of Sciences, Shanghai 201210, China; ② School of Future Technology,  University of Chinese Academy of Sciences, Beijing 100049, China; ③ Center for Transformative Science / School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210, China

Received date: 2024-03-05

  Online published: 2024-06-27

摘要

短波自由电子激光产生的从极紫外(XUV)至硬X射线范围内连续可调的超强、超快和高相干性的脉冲辐射,为研究原子、分子和团簇中的超快电子和结构动力学过程开辟了新的途径。从原子的少光子单电离、少光子多电离和多光子多电离过程,到单脉冲的分子结构成像和时间分辨的分子动力学,再到团簇中的超快能量和质子转移过程,短波自由电子激光的应用非常广泛,并且取得了一系列重大的成果。通过一些科学案例,梳理了短波自由电子激光在原子、分子和团簇领域的研究进展。最后,总结了短波自由电子激光目前在该领域取得的成就,并展望了未来发展趋势。

本文引用格式

董瑞超, 冯金泽, 王新成, 江玉海 . 短波自由电子激光在原子分子和团簇中的应用[J]. 自然杂志, 2024 , 46(3) : 203 -220 . DOI: 10.3969/j.issn.0253-9608.2024.03.005

Abstract

Short-wavelength free-electron lasers provide ultra-intense, ultra-fast, and highly coherent pulse radiation, tunable from extreme ultraviolet (XUV) to hard X-ray regimes, opening up new avenues for studying ultra-fast electron and structural dynamics processes in atoms, molecules, and clusters. From the few-photon single-ionization, few-photon multiple-ionization, and multiphoton multiple-ionization processes induced in atoms to single-pulse imaging of molecular structures and time-resolved molecular dynamics, further to ultra-fast energy and proton transfer processes in clusters, short-wavelength free-electron lasers have a wide range of applications and a number of groundbreaking achievements have successively achieved. The recent research progress of shortwavelength free-electron lasers in the field of atoms, molecules and clusters is systematically reviewed through several illustrative scientific cases. Finally, the current achievements and future development trends of short-wavelength free-electron lasers in this field are summarized and prospected.
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