自然杂志 ›› 2017, Vol. 39 ›› Issue (4): 235-241.

• 专题综述 •    下一篇

光电催化还原二氧化碳概览

饶旭峰, 许杰①②, 刘予宇①②, 张久俊①②   

  1. ①上海大学理学院,上海 200444;②上海大学可持续能源研究院,上海 200444
  • 收稿日期:2017-06-14 修回日期:2017-06-14 出版日期:2017-08-25 发布日期:2017-09-12

Photoelectrocatalysis of carbon dioxide

RAO Xufeng, XU Jie①②, LIU Yuyu①②, ZHANG Jiujun①②   

  1. ①College of Sciences, Shanghai University, Shanghai 200444, China; ②Institute of Sustainable Energy, Shanghai University,
    Shanghai 200444, China
  • Received:2017-06-14 Revised:2017-06-14 Online:2017-08-25 Published:2017-09-12

摘要:

       光电催化还原二氧化碳(CO2)利用光能和电能可以将二氧化碳转化为液体燃料或其他有机化合物,还原过程结合了光 催化还原和电化学还原的优点,具有巨大的应用潜力。通过简要介绍并比较光催化转化、电催化还原和光电协同催化还原CO2的原理和特点,得出光电催化还原CO2具备诸多优点,并对光电催化还原CO2的影响因素进行了分析,最后对其未来的 研究方向进行了展望。

关键词: 光催化, 光电催化, 二氧化碳还原

Abstract:

Photoelectrocatalysis of carbon dioxide utilizes solar power and electrical power as energy sources to convert carbon dioxide (CO2) into liquid fuels or other organic compounds. This process combines photocatalytic reduction and electrochemical reduction, and possesses great potential for future applications. In this paper, fundamental mechanisms and characteristics of photocatalysis, electrochemical reduction and photoelectrocatalysis are briefly introduced. The advantages of photoelectrocatalysis are emphasized, and the factors affecting CO2 photoelectrocatalysis are also analyzed. Future research directions on CO2 photoelectrocatalysis are then proposed.

Key words: photocatalysis, photoelectrocatalysis, carbon dioxide reduction

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